What should I upgrade first?

Neither. SATA 3 is backward compatible. Buy a sata 3 ssd and just run it through sata 2 on your motherboard. It'll run fine, just not at full sata 3 speeds, so may be like 10% slower than what it would be if you did have sata 3
 
Dammit, I can't choose between the GTX 560 Ti or HD7850 OR should I wait for the 660 Ti which is coming out soon?
 
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